Executive Summary

This report for the fourth quarter, 2001, contains results from the Environmental Surveillance, Education, and Research (ESER) Program’s monitoring of the Department of Energy’s Idaho National Engineering and Environmental Laboratory’s (INEEL) offsite environment, October 1 through December 31, 2001.  All sample types (media) and the sampling schedule followed during 2001 are listed in Appendix A.  Specifically, this report contains the results for the following:

Air Sampling

At no time during the fourth quarter were weekly average gross alpha or gross beta concentrations from Boundary locations statistically higher than corresponding averages for Distant locations, as one would expect if the INEEL was a significant source of radionuclide contamination.  During the fourth quarter, analysis of one ten-cartridge batch detected 131I greater than the associated 2s and minimum detectable concentration (MDC) values.  Immediate reanalysis of each individual cartridge yielded results below both the MDC and 2s values.  Because initial counting is done as a batch sample it appears that the cumulative activity for these ten cartridges was above the 2s/MDC value, but was not attributable to any single location (cartridge).  Selected quarterly composite filter samples were analyzed for gamma emitting radionuclides, strontium-90 (90Sr), plutonium-238 (238Pu), plutonium-239/240 (239/240Pu), and americium-241 (241Am).  Five samples showed at least one human-made radionuclide greater than its related 2s value.  All results were far less than their respective Derived Concentration Guide (DCG).  In addition, 241Am was detected in one blank sample.  Because blank samples should have no detectable radioactivity and the result was close to 2s, the result is questionable and most likely not valid.  Details of the low-volume air sampling appear in section 3.1.

Eleven atmospheric moisture samples were obtained during the fourth quarter of 2001; one from Blackfoot, two from Rexburg, and four each from Idaho Falls and Atomic City.  All sample results but one, collected from Rexburg in October, exceeded their respective 2s values.  All were well below the DCG value of 1 x 10-7 µCi/mL (3.7 x 10-3 Bq/mL) for tritium in air.  Details of atmospheric moisture sampling appear in section 3.2.

The ESER Program operates three PM10 samplers, one each at Rexburg, Blackfoot, and Atomic City.  Sampling of PM10 is informational as no analyses are conducted for contaminants.  PM10 concentrations were well below all health standard levels for all samples.  The maximum 24-hour concentration was 77.8 µg/m3 on November 11, 2001, in Blackfoot.  Details of PM10 sampling appear in section 3.3.

Precipitation Sampling

Sufficient precipitation occurred to allow collection of three monthly composite samples each from Idaho Falls and from the Central Facilities Area (CFA) on the INEEL, and six weekly samples from the Experimental Field Station (EFS) on the INEEL.  Tritium was detected in nine samples: two from Idaho Falls, three from CFA, and four from EFS.  There is no DCG for tritium in precipitation, but in drinking water it is 80,000 pCi/L (2,960 Bq/L).  The Safe Drinking Water Act sets a limit of 20,000 pCi/L (740 Bq/L) for tritium.  The levels of tritium measured in fourth quarter precipitation samples were well below the DCG value and the Safe Drinking Water Act Limit.  Details of precipitation sampling appear in section 4.1.

Drinking Water Sampling

Drinking water samples were collected from tap water from 14 locations throughout southeast Idaho.  All were analyzed for gross alpha, gross beta, and tritium.  Three drinking water samples had a gross alpha results greater than their associated 2s values.  Eleven of the 14 drinking water samples had gross beta results greater than their associated 2s values.  The DCG values for gross alpha and gross beta in water are 30 pCi/L and 100pCi/L, respectively.  The EPA has set the limits for gross alpha and gross beta in water at 15 pCi/L and 50 pCi/L, respectively.  The maximum gross alpha result, in the sample from Monteview, was many times lower than the DCG value and the Safe Drinking Water Act limit.  Gross beta concentrations in all fourth quarter drinking water samples were also at least nine times lower than the DCG value and four times lower than the Safe Drinking Water Act limit.  Gross alpha and beta concentrations were not higher at locations “down stream” from the INEEL.  Tritium analyses showed seven drinking water samples with a result greater than their 2s value.  The maximum result from the Idaho Falls sample result was much lower than the DCG value and the Safe Drinking Water Act Limit.  Details of drinking water sampling appear in section 4.2.

Surface Water Sampling

Surface water samples were collected from five locations along the Snake River in the area where the Snake River Plain Aquifer discharges and from one upstream location in Idaho Falls.  Samples were analyzed for the same constituents as drinking water.  No sample had detectable concentrations of gross alpha activity.  All samples had detectable levels of gross beta activity, which did not exceed the DCG and SDWA limit and were well within the range of past measurements.  One sample, collected at Hagerman, had a detectable concentration of tritium, well within results measured in the past.  The tritium result was far less than the DCG and SDWA limit for tritium in drinking water.  Details of surface water sampling appear in section 4.3.

Milk Sampling

Milk samples were collected weekly in Idaho Falls and monthly at eight other locations around the INEEL.  All samples were analyzed for gamma emitting radionuclides with samples from four locations (Arco, Dietrich, Howe, and Roberts) being analyzed for 90Sr.  Iodine-131 was detected in two samples, one from Roberts and one from Idaho Falls.  However, reanalysis of these samples indicated no detectable levels of 131I. Three samples had 137Cs concentrations greater than their 2s uncertainty.  Of the four samples analyzed for 90Sr only the Arco sample did not yield concentrations greater than their associated 2s value.  There are no established limits for 137Cs or 90Sr in milk but, for comparison, the EPA has set the limit for 137Cs in drinking water at 12 pCi/L and at 8pCi/L for 90Sr.  The Safe Drinking Water limit is based on a 4 mrem per year maximum allowable dose and the assumption that two liters per day are consumed.  The maximum 137Cs concentration measured in milk during the fourth quarter, 2001 was many times lower than the 12 pCi/L limit and the maximum 90Sr concentration was below the 8 pCi/L limit.  Details of milk sampling appear in section 5.1.

Game Animal Sampling

Three large game animals were sampled during the fourth quarter of 2001.  All were killed as a result of vehicular collisions.  These accidents all involved mule deer (Odocoileus hemionus).  Thyroid, liver, and muscle tissue were collected from each animal.  None of the samples contained measurable radionuclides above the 2s uncertainty or the MDC.  Details of large game animal sampling appear in section 5.2.

Potato Sampling

Potatoes were collected from various growers in southeast Idaho as well as from locations around the United States.  All samples were analyzed for gamma emitting radionuclides and 90Sr.  No sample collected during the fourth quarter contained levels of 90Sr or 137Cs above the 2s level.  Details of potato sampling appear in section 5.3.

Waterfowl Sampling

Fourteen waterfowl were collected during 2001: three each from the Idaho Nuclear Technology and Engineering Center (INTEC) percolation ponds and Market Lake and four each from the Argonne National Laboratory-West (ANL-W) and Test Reactor Area (TRA) ponds.  All were analyzed for gamma emitting radionuclides with a subset analyzed for 90Sr, plutonium-238 (238Pu), plutonium‑239/240 (239/240Pu), and americium-241 (241Am).  Seven ducks had detectable levels of at least one radionuclide in edible tissue.  The highest concentrations were in the TRA samples.  Duck hunting is not allowed on the INEEL but a maximum potential exposure scenario to humans would be someone collecting a duck directly from the TRA radioactive waste ponds and immediately consuming all muscle, liver, heart, and gizzard tissue.  The estimated dose, 0.08 mrem, is far less than the dose limit of 100 mrem.  Details of duck sampling appear in section 5.4.

Direct Radiation

The ESER and its predecessors have placed an array of thermoluminescent dosimeters (TLDs) throughout the Eastern Snake River Plain to measure the amount of radiation in the environment.  The results of the November sampling (the period of measurement being May 2001 through November 2001) show the average exposure rate for locations in the Boundary group to range from a low of 0.32 mR/day at Birch Creek to a high of 0.40 mR/day at Mud Lake.  The overall average was 0.35 mR/day.  The Distant set had a high of 0.43 mR/day at Rexburg and a low of 0.33 mR/day at the new station in Jackson Wyoming.  The overall average Distant value was 0.36 mR/day.  There was no statistical difference between Boundary and Distant locations.  Details of environmental radiation measurements appear in section 6.

Conclusions

Overall, the only radionuclides measured that could be attributed to the INEEL were 60Co and 137Cs in some of the ducks and doves collected directly from contaminated waste ponds on the INEEL.  No radionuclides in any other samples taken during the fourth quarter, 2001, could be directly linked with INEEL activities.  Levels of detected radionuclides were below regulatory limits and not different from values measured at other locations across the United States.  Concentrations of 60Co and 137Cs in ducks from TRA were higher than in samples taken from offsite locations, still, all concentrations were much lower than regulatory dose limits.  Concentrations in all of the samples collected and analyzed during the fourth quarter, 2001 were below guidelines set by both the DOE and the U.S. Environmental Protection Agency (EPA) for protection of the public.

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